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Effect of phonon bath dimensionality on the spectral efficiency of single-photon emitters in the Purcell regime

机译:声子浴维数对光谱效率的影响   purcell制度中的单光子发射器

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摘要

We develop a theoretical frame to investigate the single-photon emissionspectral efficiency of a solid-state nano-emitter embedded in a high qualityfactor micro-cavity. This study encompasses the case of localized excitonsembedded in a one, two or three-dimensional matrix. The populations evolutionsare calculated based on a spin-boson model, using the non-interacting blipapproximation (NIBA). We find that the single-photon spectral efficiency of thecavity-coupled emitter can be expressed by a simple formula, taking as inputsthe free-space emission and absorption spectra of the emitter as well as theloss rates of the system. In other words, the information on the interactionbetween the exciton and the phonon bath, encoded in the free-space behavior ofthe emitter, is sufficient to obtain the dynamics of the system in the cavity.We compute numerically the spectral efficiency for several types of localizedemitters and show distinct behaviors depending on the phonon bathdimensionality. In particular, a pronounced asymmetric energy exchange betweenthe emitter and the cavity on the side-bands can yield a considerable extensionof the tuning range of the sources through phonon-assisted cavity feeding.
机译:我们开发了一个理论框架,以研究嵌入在高品质因数微腔中的固态纳米发射体的单光子发射光谱效率。这项研究涵盖了嵌入在一维,二维或三维矩阵中的局部激子的情况。使用无相互作用的Blipapproximation(NIBA),基于自旋玻色子模型计算种群进化。我们发现腔耦合发射器的单光子光谱效率可以用一个简单的公式表示,将发射器的自由空间发射和吸收光谱以及系统的损耗率作为输入。换句话说,关于激子和声子浴之间相互作用的信息,以发射体的自由空间行为进行编码,足以获得腔体内系统的动力学。我们通过数值计算了几种局部发射体的光谱效率并表现出不同的行为,具体取决于声子浴维数。特别地,在发射器和边带上的腔之间的明显的不对称能量交换可以通过声子辅助的腔馈送而显着扩展源的调谐范围。

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